Efficient generation of nonlinear phenomena related to third order optical non-linear susceptibility Χ(3) interactions in triply resonant silica microspheres is presented in this paper. The interactions here reported are: Stimulated Raman Scattering (SRS), and four wave mixing processes comprising Stimulated Anti-stokes Raman Scattering (SARS).
Farnesi, D., Berneschi, S., Cosi, F., Righini, G. C., Soria, S., Nunzi Conti, G. Stimulated Stokes and Antistokes Raman Scattering in Microspherical Whispering Gallery Mode Resonators. J. Vis. Exp. (110), e53938, doi:10.3791/53938 (2016).